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Anisotropy of Antiferromagnetic 180[degree] Domains in LiCoPO[sub 4] and LiNiPO[sub 4] Export

Physical Review Letters, Vol. 101, No. 15. (2008), 157202.

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antiferromagnetism domains licopo4 linipo4

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Unexpected three-dimensional distributions of antiferromagnetic 180° domains are observed in LiCoPO4 and LiNiPO4 by optical second harmonic generation. Domains in LiCoPO4 are isotropic in spite of the quasi-two-dimensional magnetic structure whereas domains in LiNiPO4 are distinctly anisotropic, but in contrast to the anisotropy of the magnetic structure. The diversity reveals a potential for fine-tuning magnetic properties determined by the distribution of domains or domain walls and the urgent need for an improved understanding of spatial correlations in antiferromagnets.


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