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Time-Resolved X-Ray Diffraction from Coherent Phonons during a Laser-Induced Phase Transition Export

Physical Review Letters, Vol. 84, No. 1. (3 January 2000), 111.

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coherent laser-induced phonons plase-transitions txrd

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Time-resolved x-ray diffraction with picosecond temporal resolution is used to observe scattering from impulsively generated coherent acoustic phonons in laser-excited InSb crystals. The observed frequencies and damping rates are in agreement with a model based on dynamical diffraction theory coupled to analytic solutions for the laser-induced strain profile. The results are consistent with a 12 ps thermal electron-acoustic phonon coupling time together with an instantaneous component from the deformation-potential interaction. Above a critical laser fluence, we show that the first step in the transition to a disordered state is the excitation of large amplitude, coherent atomic motion.


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