Multiphoton Intrapulse Interference. 1. Control of Multiphoton Processes in Condensed Phases Export

@article{citeulike:1595401, abstract = {Abstract: We explore and demonstrate the use of phase-modulated ultrafast laser pulses for controlling nonlinear optical processes in large molecules, proteins, and solid materials. Our experiments illustrate that in condensed phases, when spectra are broad, the spectrum of the nth-order electric field, determined by multiphoton intrapulse interference, plays a major role in controlling multiphoton excitation. These findings determine key parameters (amplitude, period, and symmetry of the phase function) for coherent femtosecond laser control in condensed phases.}, address = {Department of Chemistry and Department of Physics and Astronomy, Michigan State University, East Lansing, Michigan 48824}, author = {Walowicz, K. A. and Pastirk, I. and Lozovoy, V. V. and Dantus, M.}, citeulike-article-id = {1595401}, citeulike-linkout-0 = {http://dx.doi.org/10.1021/jp0258964}, citeulike-linkout-1 = {http://pubs.acs.org/doi/abs/10.1021/jp0258964}, day = {17}, doi = {10.1021/jp0258964}, journal = {J. Phys. Chem. A}, keywords = {coherent, control}, month = {October}, number = {41}, pages = {9369--9373}, posted-at = {2008-03-17 21:13:06}, priority = {2}, title = {Multiphoton Intrapulse Interference. 1. Control of Multiphoton Processes in Condensed Phases}, url = {http://dx.doi.org/10.1021/jp0258964}, volume = {106}, year = {2002} }

TY - JOUR ID - citeulike:1595401 L3 - citeulike-article-id:1595401 N2 - Abstract: We explore and demonstrate the use of phase-modulated ultrafast laser pulses for controlling nonlinear optical processes in large molecules, proteins, and solid materials. Our experiments illustrate that in condensed phases, when spectra are broad, the spectrum of the nth-order electric field, determined by multiphoton intrapulse interference, plays a major role in controlling multiphoton excitation. These findings determine key parameters (amplitude, period, and symmetry of the phase function) for coherent femtosecond laser control in condensed phases. IS - 41 JF - J. Phys. Chem. A AD - Department of Chemistry and Department of Physics and Astronomy, Michigan State University, East Lansing, Michigan 48824 EP - 9373 TI - Multiphoton Intrapulse Interference. 1. Control of Multiphoton Processes in Condensed Phases VL - 106 SP - 9369 KW - coherent KW - control AU - Walowicz, KA AU - Pastirk, I AU - Lozovoy, VV AU - Dantus, M PY - 2002/10/17/ UR - http://dx.doi.org/10.1021/jp0258964 ER -