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Growing Spatial Correlations of Particle Displacements in a Simulated Liquid on Cooling toward the Glass Transition Export

Physical Review Letters, Vol. 82, No. 25. (21 Jun 1999), pp. 5064-5067.

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We define a correlation function that quantifies the spatial correlation of single-particle displacements in liquids and amorphous materials. We show that for an equilibrium liquid this function is related to fluctuations in a bulk dynamical variable. We evaluate this function using computer simulations of an equilibrium glass-forming liquid; and show that long range spatial correlations of displacements emerge and grow on cooling toward the mode coupling critical temperature.


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