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Infrared optical absorption spectra of CuO single crystals: Fermion-spinon band and dimensional crossover of the antiferromagnetic orderPhysical Review B (Condensed Matter and Materials Physics), Vol. 80, No. 14. (2009), 140516.
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AbstractWe have obtained mid-infrared optical absorption spectra of the S=1/2 quasi-one-dimensional CuO using polarized transmission measurement and interpreted the spectra in terms of phonon-assisted magnetic excitations. When the electric field is parallel to the main antiferromagnetic direction a shaped peak is observed with the maximum at =0.23 eV which is attributed to spinons along Cu-O chains. At low temperatures in the antiferromagnetic phase another peak appears at =0.16 eV which is attributed to two-magnon absorption but the spinon peak remains. This behavior is interpreted as due to a dimensional crossover where the low-temperature three-dimensional magnetic phase keeps short-range characteristics of a one-dimensional magnet.
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