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Time-resolved pump-probe experiments beyond the jitter limitations at FLASH Export

Applied Physics Letters, Vol. 94, No. 14. (7 April 2009), 144102.

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arrival bunch electron electro-optic femtosecond laser measurement probe pump synchronization time tisa

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Using a noninvasive, electro-optically based electron bunch arrival time measurement at FLASH (free electron laser in Hamburg) the temporal resolution of two-color pump-probe experiments has been significantly improved. The system determines the relative arrival time of the extended ultraviolet pulse of FLASH and an amplified Ti:sapphire femtosecond-laser pulse at the interaction region better than 90 fs rms. In a benchmarking pump-probe experiment using two-color above threshold ionization of noble gases, an enhancement in the timing resolution by a factor of 4 compared to the uncorrected data is obtained.


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